Ortho-carbaborane derivatives of indomethacin as cyclooxygenase (COX)-2 selective inhibitors.

Authors

Scholz M Matthias , Blobaum AL Anna L , Marnett LJ Lawrence J , Hey-Hawkins E Evamarie .
Bioorganic & medicinal chemistry. 2012 8 1; 20(15).
4830-7

Abstract

A series of novel indomethacin analogues with carbaboranes as three-dimensional substitutes for the chlorophenyl ring have been prepared. Their cyclooxygenase (COX) inhibition and enzyme selectivity has been tested and compared to the corresponding adamantyl analogues. Surprisingly, only the ortho-carbaborane derivatives were active compounds. Preliminary biological studies gave an interesting insight into the validity of employing carbaboranes as pharmacophores.

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